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Spurlock had a total of 23 receptions for 200 yards and a touchdown in 2012 for San Diego. He also was the primary kick and punt returner by the end of the season.
Spurlock did not catch a pass Sunday against the Jets, but he handled all of the punt and kick returns and notched a 63-yard punt return touchdown.
Spurlock agreed to a contract with the Jaguars on Friday, according to the team's official Twitter page.
Spurlock signed with the Chargers on Wednesday, Michael Gehlken of the San Diego Union-Tribune reports.
Spurlock finished the 2011 season with two receptions for 13 yards, six punt returns for 21 yards and two kick returns for 33 yards in 12 games played.
Spurlock will sign his tender from the Bucs on Friday, according to Anwar Richardson of the Tampa Tribune.